Year

2018

Type(s)

Journal Article

Author(s)

Higginbotham, H.F. and Pander, P. and Rybakiewicz, R. and Etherington, M.K. and Maniam, S. and Zagorska, M. and Pron, A. and Monkman, A.P. and Data, P.

Source

Journal of Materials Chemistry C, 6(30): 8219—8225, 2018

Url

https://www.scopus.com/inward/record.uri?eid=2-s2.0-85051092011&doi=10.1039%2fc8tc02936a&partnerID=40&md5=4d8bcaed94ae8fd553040f018ad9b0b1

BibTeX

BibTeX

BibTeX

@ARTICLE{Higginbotham20188219, author={Higginbotham, H.F. and Pander, P. and Rybakiewicz, R. and Etherington, M.K. and Maniam, S. and Zagorska, M. and Pron, A. and Monkman, A.P. and Data, P.}, title={Triphenylamine disubstituted naphthalene diimide: Elucidation of excited states involved in TADF and application in near-infrared organic light emitting diodes}, journal={Journal of Materials Chemistry C}, year={2018}, volume={6}, number={30}, pages={8219-8225}, doi={10.1039/c8tc02936a}, note={cited By 6}, url={https://www.scopus.com/inward/record.uri?eid=2-s2.0-85051092011&doi=10.1039%2fc8tc02936a&partnerID=40&md5=4d8bcaed94ae8fd553040f018ad9b0b1}, affiliation={Physics Department, Durham University South Road, Durham, DH1 3LE, United Kingdom; Cardinal Stefan Wyszynski University in Warsaw, Faculty of Mathematics and Natural Sciences, School of Exact Sciences, Wóycickiego 1/3, Warsaw, 01-938, Poland; School of Chemistry, Monash University, Clayton, VIC, Australia; Faculty of Chemistry, Warsaw University of Technology, Noakowskiego 3, Warsaw, 00-664, Poland; Faculty of Chemistry, Silesian University of Technology, Ks. M. Strzody 9, Gliwice, 44-100, Poland; Centre of Polymer and Carbon Materials, Polish Academy of Sciences, M. Curie-Sklodowskiej 34, Zabrze, 41-819, Poland}, abstract={It is demonstrated that a naphthalene diimide core disubstituted with triphenylamine can be used as a thermally activated delayed fluorescence emitter in organic light emitting diodes. Detailed spectroscopic studies demonstrated unusual host effects on the photophysical properties of this material. In particular, we were able to deduce recombination pathways and the role of the host and temperature in increasing/decreasing the TADF contribution in overall emission. Furthermore, stemming from these host effects on the geometry of the emitter we discover different local triplet states involved in the TADF mechanism. We elucidate this confusing situation to show that simply measuring low-temperature phosphorescence does not always give the energy of the local triplet involved in TADF. The studies carried out in a non-polar polymer and the OLED host were completed by NIR OLED fabrication showing promising characteristics. © 2018 The Royal Society of Chemistry.}, keywords={Fluorescence; Infrared devices; Naphthalene; Spectroscopic analysis; Temperature, Low temperatures; Naphthalene diimide; Near Infrared; Photophysical properties; Spectroscopic studies; Thermally activated delayed fluorescences; Triphenyl amines; Triplet state, Organic light emitting diodes (OLED)}, funding_details={European CommissionEuropean Commission, EC}, funding_text 1={P. P. thanks to the European Union for financial support from H2020-MSCA-ITN-2015/674990 EXCILIGHT grant. A. P. and M. Z. wish to acknowledge financial support from the National Science Centre, Poland, (NCN) Grant No. 2015/17/B/ST5/00179. P. D. acknowledges the EU’s Horizon 2020 for funding the ORZEL project under grant agreement No. 691684. H. H. and M. K. 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Adv., 3, p. e1603282}, correspondence_address1={Higginbotham, H.F.; Physics Department, Durham University South RoadUnited Kingdom}, publisher={Royal Society of Chemistry}, issn={20507534}, coden={JMCCC}, language={English}, abbrev_source_title={J. Mater. Chem. C}, document_type={Article}, source={Scopus},